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All Journal IPTEK Journal of Proceedings Series Jurnal Pendidikan IPA Indonesia Alchemy Jurnal Penelitian Kimia Indonesian Journal of Chemistry Jurnal Saintek Lahan Kering Molekul: Jurnal Ilmiah Kimia
Reinner Ishaq Lerrick
Department of Chemistry, Faculty of Science and Engineering, University of Nusa Cendana, Jl. Adi Sucipto, Penfui-Kupang 85118, NTT, Indonesia
Agriculture, Biological Sciences & Forestry Biochemistry, Genetics & Molecular Biology Chemical Engineering, Chemistry & Bioengineering Chemistry Computer Science & IT Education Energy Environmental Science Materials Science & Nanotechnology Public Health

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Journal : Indonesian Journal of Chemistry

 1 
T-grafting BODIPY-Based Photosensitizers: The Synthesis of 2,6-Diethylacrylic-8-(o-methoxyphenyl)BODIPY and Its DSSC Performance Reinner Ishaq Lerrick; Wastiana Bere; Meliana Da Silva Braga; Agus Supriyanto; Ali Hashem Essa
Indonesian Journal of Chemistry Vol 23, No 1 (2023)
Publisher : Universitas Gadjah Mada

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.22146/ijc.76919

Abstract

A new T-grafting photosensitizer of Dye-Sensitized Solar Cell (DSSC) has been developed by aligning Donor-Acceptor (D-A) group in an axially chiral BODIPY. Synthesis of the dye was conducted over a linear approach involving one-pot, non-oxidative synthesis of 1,3,5,7-tetramethyl-8-(o-methoxyphenyl)BODIPY, bromination, and finally C2/C6 ethyl acrylate Pd-Heck coupling to produce 65% of 2-ethylacrylic-1,3,5,7-tetramethyl-8-(o-methoxyphenyl)BODIPY (BOD-8) and 35% of 2,6-diethylacrylic-1,3,5,7-tetramethyl-8-(o-methoxyphenyl)BODIPY (BOD-9), both characterized by the appearance of acrylic alkenes at 6.05, and 7.63 ppm for BOD-8, and the additional 5.43, 7.80 ppm doublet peaks for BOD-9. The resulting dye showed excellent photon harvesting-related photovoltaic properties and electronic injection and regeneration processes where the acrylic esters were found to be the Donor and the aryl was the Acceptor. Eventually, the dye produced a current at 0.5% efficiency, similar to the horizontal D-A DSSC photosensitizer design.
Co-Authors Agus Supriyanto Ali Hashem Essa Chairil Anwar Debora Ratu Jumina Jumina Mariti, F. Maulidan Firdaus Meliana Da Silva Braga Parikesit, A. A. Pius Dore Ola Rensy A. Henci Saudale, F. Z. Sherlly Ledoh Theo Da Cunha Wastiana Bere Yoktan E Buraen