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All Journal International Journal of Applied Power Engineering (IJAPE) TELKOMNIKA (Telecommunication Computing Electronics and Control)
Le Doan Duy
Vinh Long University of Technology Education
Computer Science & IT Electrical & Electronics Engineering

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Investigation of the photoluminescence properties of quantum dots using theoretical simulation Le Doan Duy; Le Xuan Thuy
International Journal of Applied Power Engineering (IJAPE) Vol 15, No 2: June 2026
Publisher : Institute of Advanced Engineering and Science

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.11591/ijape.v15.i2.pp942-947

Abstract

This study investigates the optical behavior of CdSe quantum dots, a class of semiconductor nanomaterials widely studied for light-emitting, photovoltaic, and bioimaging applications owing to their size-dependent electronic structure. The objective is to clarify the relationship between quantum dot size, size distribution, and emission characteristics through experimental and simulated optical spectra. UV-Vis absorption, photoluminescence, and simulated PL spectra were analyzed for CdSe quantum dots excited at 325 nm. The experimental PL spectrum exhibits a single and narrow emission band assigned to the 1Se → 1Sh transition, which is blue-shifted compared with bulk CdSe, confirming strong quantum confinement in 2-3 nm particles with a very narrow size distribution of less than 1%. A large Stokes shift of 0.93 eV is observed, attributed to confinement effects and surface-related states. Simulated photoluminescence (PL) spectra for 3-6 nm quantum dots show progressive red-shifting and spectral broadening with increasing particle size, while smaller quantum dots display stronger PL intensity due to enhanced confinement and more efficient radiative recombination. Parameter analysis further reveals that size deviation and linewidth broaden emission and reduce intensity without changing the peak wavelength. These findings provide useful guidance for optimizing CdSe quantum dots for QLEDs, bioimaging, and broadband optoelectronic devices.
Synthesis of reduced graphene oxide decotate Cu2S nanoparticles for cathode of quantum dot solar cell Le Doan Duy; Le Thi Ngoc Tu; Le Tien Dat
TELKOMNIKA (Telecommunication Computing Electronics and Control) Vol 22, No 1: February 2024
Publisher : Universitas Ahmad Dahlan

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.12928/telkomnika.v22i1.25238

Abstract

In this paper, the results of making a reduced graphene oxide cathode electrode with Cu2S nanoparticles are shown so that it can be used as a counter electrode in quantum dot solar cells to replace other counter electrodes. An rGO-Cu2S paste obtained by hydrolysis was scanned onto the surface of the fluorine-doped tin oxide (FTO) conductive substrate when bound to Cu2S nano by a screen-printing process, then calcined at 350 °C to crystallize the film. Following calcination, the film was examined for structure using energy-dispersive X-ray (EDX) and X-ray diffraction (XRD) spectroscopy, as well as for type and particle size using scanning and transmission electron microscopy and transmission electron microscopy, respectively. Mott-schottky measurement is used to determine the semiconductor and carrier concentrations in the film, and an electrochemical device is used to assess the electrodes redox capacity in a polysulfide electrolyte solution. The operability of the rGO-Cu2S cathode at the peak of the current density in the C-V curve was 24 mA/cm2, a 30-fold increase compared to that of the Cu2S electrode. This result shows that the efficiency, Voc, FF, Jsc are 4.92%, 0.525 V, 0.418, and 22.4 mA/cm2, respectively.
Co-Authors Le Thi Ngoc Tu Le Tien Dat Le Xuan Thuy