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Neza Rahayu Palapa
Graduate School, Faculty of Mathematics and Natural Sciences, Sriwijaya University, Palembang, 30139, Indonesia
Biochemistry, Genetics & Molecular Biology Chemical Engineering, Chemistry & Bioengineering Environmental Science Materials Science & Nanotechnology Physics

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ZnAl-Humic Acid Composite as Adsorbent of Cadmium(II) From Aqueous Solution Jeri Rahmadan; Veronika Parhusip; Neza Rahayu Palapa; Tarmizi Taher; Risfidian Mohadi; Aldes Lesbani
Science and Technology Indonesia Vol. 6 No. 4 (2021): October
Publisher : Research Center of Inorganic Materials and Coordination Complexes, FMIPA Universitas Sriwijaya

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.26554/sti.2021.6.4.247-255

Abstract

The modified ZnAl composites with humic acid (HA/ZnAl composite) were a coprecipitation method used as an adsorbent to remove cadmium(II) in an aqueous solution. The synthesized material was characterized using SEM-EDX, FTIR, and XRD. From the analysis using XRD, there is a widening peak at an angle of 2???? (24°), FTIR analysis there is a new peak at 1000 cm−1 and 1220 cm−1 and SEM analysis show that there is a change in surface morphology due to more aggregated particles. The experimental results on HA/ZnAl composite followed the PSO model, where the cadmium(II) removal process was chemical adsorption. The adsorption isotherm follows the Langmuir model where adsorption occurs in a monolayer and maximum adsorption capacity was obtained 38.76 mg/g higher than pristine. Thermodynamics of the adsorption process of cadmium(II) in an aqueous solution occurred spontaneously where G < 0 at all temperatures and endothermic properties were tested. The performance of the HA/ZnAl composite showed that strong potential as an adsorbent of low cost, high efficiency, easy operation, and good reusability. The cadmium(II) was absorbed on the surface of HA/ZnAl composite by surface complexation and chelating interactions, and surface complexation was the main route of cadmium(II) removal. In addition, HA/ZnAl composite has excellent treatment efficiency in actual aqueous solution.
Co-Authors Aldes Lesbani Jeri Rahmadan Risfidian Mohadi Tarmizi Taher Veronika Parhusip