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All Journal Jurnal Teknik ITS IPTEK The Journal of Engineering MEKANIKA - JURNAL TEKNIK MESIN Journal of Energy, Material, and Instrumentation Technology Jurnal Nasional Aplikasi Mekatronika, Otomasi dan Robot Industri (AMORI) Sewagati
Ahmad Fauzan Adziimaa
Institut Teknologi Sepuluh Nopember
Arts Humanities Chemical Engineering, Chemistry & Bioengineering Civil Engineering, Building, Construction & Architecture Control & Systems Engineering Education Electrical & Electronics Engineering Energy Engineering Languange, Linguistic, Communication & Media Materials Science & Nanotechnology Mechanical Engineering Physics Public Health Social Sciences Other

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Exponential-Offset Modelling and XRD Correlation of SOH Degradation in LiFePO4 Batteries under Extreme Loading Latif, Chaironi; Maulana, Tubagus Adam Jody; Yogianto, Mohammad Fahmi Ilmi; Adziimaa, Ahmad Fauzan
Journal of Energy, Material, and Instrumentation Technology Vol 6 No 4 (2025): Journal of Energy, Material, and Instrumentation Technology (In Press)
Publisher : Departement of Physics, Faculty of Mathematics and Natural Sciences, University of Lampung

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.23960/jemit.379

Abstract

Understanding the relationship between electrochemical degradation and structural changes is critical for improving the reliability of lithium-ion batteries. In this study, the state of health (SOH) of 18650-type lithium iron phosphate (LiFePO4, LFP) cells was evaluated under extreme loading using discharge resistances of 2.5 Ω and 0.005 Ω. The SOH decreased sharply after the first cycle and then declined more gradually, and the degradation trend was well described by an exponential-offset model with RMSE = 2.87, MAE = 2.25, and R2 = 0.90. Structural analysis was performed by X-ray diffraction (XRD) on electrode samples taken after one discharge at 2.5 Ω (L1), 100 discharges at 2.5 Ω (L100), and one discharge at 0.005 Ω (LD). The XRD results confirmed that the main phase was graphite, but with reduced peak intensities, peak broadening, and increased background noise, indicating crystallinity loss and partial amorphization. These findings demonstrate that SOH degradation is strongly correlated with the decline in crystallinity, and that extreme loading can trigger significant structural deterioration even within a single discharge.
Co-Authors Anggun, Adinda Anida Oktavia Rachmadianti Anida Oktavia Rachmadianti Avicenna, Ruci Azizah, Salma Chaironi Latif Danang Adi, Danang Detak Yan Pratama Dewi Sugihartati Elda Yofi Pramadani Fadilah, Davan Ilham Kurniawan Imah Luluk Kusminah Isa Hafidz Izzan, M. Maulana, Tubagus Adam Jody Mukti, Ilham Hary Nabila Widad Dira Sinatrya Nurisalam, Royhan Patrialova, Sefi Novendra Pramadani, Elda Yofi Rachmadi, Rahadiyan Rahmat, Nugie Risyad, Ibrahim Rozak, M. Abdul Safira Firdaus Mujiyanti Saifullah, Ahmad Wahyu Nur Handayani Wahyudi, Ibnu Ari Yogianto, Mohammad Fahmi Ilmi Zakky, Ahmad