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All Journal Chimica et Natura Acta ASEAN Journal of Community Engagement Makara Journal of Science Molekul: Jurnal Ilmiah Kimia Environmental and Materials
Syauqi, Muhammad Iqbal
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Agriculture, Biological Sciences & Forestry Biochemistry, Genetics & Molecular Biology Chemical Engineering, Chemistry & Bioengineering Chemistry Control & Systems Engineering Economics, Econometrics & Finance Education Energy Engineering Environmental Science Materials Science & Nanotechnology Physics Public Health Social Sciences Other

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Journal : Makara Journal of Science

 1 
Comparative Study of Bismuth Ferrite Deposition Method on TiO2 Nanotube and Performance of Hydrogen Evolution in a Photoelectrochemical Dye-Sensitized Solar Cell Tandem System Yunita, Yunita; Syauqi, Muhammad Iqbal; Gunlazuardi, Jarnuzi
Makara Journal of Science
Publisher : UI Scholars Hub

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Hydrogen is a renewable and environmentally friendly energy source that can replace fossil fuels by utilizing solar energy through water splitting. The hydrogen production was conducted in this research by using a tandem system of dye-sensitized solar cell–photoelectrochemical cell (DSSC–PEC) and a TiO2 nanotube coated with BiFeO3 (BiFeO3/TNT) as a photoanode in the PEC. The deposition of BiFeO3 on TNT was prepared using the following three methods: successive ionic layer adsorption and reaction (SILAR), ultrasonication-assisted SILAR, and ultrasonic– immersion method by varying the number of deposition cycles in each method. In this study, the optimum cycles for SILAR, ultrasonication-assisted SILAR, and ultrasonic–immersion methods were 15, 5, and 3, respectively. Results show that the BiFeO3 deposited on TNT using the ultrasonic–immersion method with three cycles (BiFeO3/TNT_UI3) demonstrates the best photoelectrochemical activity. The tandem system comprises BiFeO3/TNT_UI3 photoanode and Pt-coated TNT dark cathode PEC cell connected to TNT/N719-based DSSC with an efficiency of 1.27%. The constructed DSSC–PEC system could produce 3.11 × 10−6 mol hydrogen in 6 h with a solar-to-hydrogen (STH) efficiency of 0.0033% in an H-type reactor filled with 0.5 M H2SO4 electrolyte.
TiO2 Crystallization at Room Temperature and Preparation of Transparent Carbon Counter Electrode for Low-Cost Dye-Sensitized Solar Cells Syauqi, Muhammad Iqbal; Sanjaya, Afiten Rahmin; Madiabu, Mohammad Jihad; Khalil, Munawar; Gunlazuardi, Jarnuzi
Makara Journal of Science Vol. 27, No. 2
Publisher : UI Scholars Hub

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We developed a low-cost dye-sensitized solar cell (DSSC) using TiO2 fabricated via rapid breakdown anodization (RBA) and ultrafast room-temperature crystallization (URTC). The prepared TiO2 was deposited on a self-made fluorine-doped tin oxide (FTO) conductive glass, and the FTO/TiO2 system was sensitized using curcumin dye. The DSSC was constructed by sandwiching the FTO/TiO2/curcumin electrode with an I−/I2 electrolyte and a transparent carbon counter electrode prepared using a liquid–liquid interface system. The characterization results showed that the TiO2 freshly prepared via URTC was transformed into an anatase crystalline phase, which exhibited a 3.10 eV band gap and a 10.08 nm average crystallite size, comparable to those of the TiO2 prepared via the conventional 450 °C annealing treatment (3.13 eV, 11.60 nm). The photocurrent activity of the URTC-prepared TiO2 under ultraviolet light (0.10 mA/cm2) was also comparable to that of the annealed TiO2 (0.12 mA/cm2). In addition, a transparent carbon electrode (FTO/Ct) was prepared successfully; it exhibited a ±58.26% transparency under visible light and comparable electrocatalytic activity to Pt-coated FTO. The DSSC based on FTO/TiO2-URTC/curcumin and FTO/Ct showed front and back illumination efficiencies of 0.47% and 0.26%, respectively. These results are only slightly lower than those of the conventional DSSC with FTO/annealed TiO2/curcumin//FTO/Pt, which exhibited front and back illumination efficiencies of 0.52% and 0.36%, respectively.
Co-Authors Adriana, Elva Dissa Agustino Zulys Arda, Hany Dwi Bambang Heru Susanto, Bambang Heru Cahyani, Annisa Titi Haidir, Banu Muhammad Istiqomah, Muhsinatul Jarnuzi Gunlazuardi Madiabu, Mohammad Jihad Munawar Khalil Prastika Krisma Jiwanti Putri, Yulia Mariana Tesa Ayudia RAHMAT WIBOWO Sanjaya, Afiten Rahmin Sherly Kasuma Warda Ningsih Utami, Chichi Amne Yunita Yunita