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Greensusmater
Published by Green and Sustainable Materials Society
ISSN : -     EISSN : 3047910X     DOI : https://doi.org/10.62755/
Core Subject : Science, Social, Engineering,
Chemical Engineering, Chemistry & Bioengineering Chemistry Environmental Science Materials Science & Nanotechnology
Greensusmater is a premier, gold open access peer-reviewed academic journal dedicated to advancing knowledge and understanding of green and sustainable materials science and technology. Our aim is to serve as a global platform for researchers, industry professionals, policymakers, and anyone interested in development of green and sustainable materials, to share their insights, discuss theories, and promote environmentally-responsible practices in materials science. We also aim to inspire collaboration, stimulate new ideas, and facilitate the practical application of research findings towards a greener and more sustainable world. In its first inaugural year, Greensusmater will publish two issues within a single volume, with releases in February and July, establishing a biannual publication rhythm.
Arjuna Subject : Ilmu Material (semua kategori) - Ilmu Material (Lain-Lain)
Articles 27 Documents
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Niobium oxide electrode performance boosted by molybdenum doping and calcination for supercapacitor applications Al Mubarok, Muhammad Ramadhan; Nurfitria, Rima; Aflaha, Rizky; Nurfani, Eka; Rianjanu, Aditya
Greensusmater Vol. 2 No. 2 (2025)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/greensusmater.2025.2.2.62-69

Abstract

Niobium pentoxide (Nb2O5) is a promising pseudocapacitive material for supercapacitor applications due to its high theoretical capacitance and electrochemical stability. However, its practical performance is limited by low electrical conductivity and poor ion transport kinetics. In this work, we report the enhancement of Nb2O5 electrode performance through molybdenum (Mo) doping and thermal calcination. Mo-doped Nb2O5 nanostructures were synthesized via a hydrothermal method followed by calcination at 500 °C. Scanning electron microscopy (SEM) and energy-dispersive X-ray spectroscopy (EDS) confirmed a rougher morphology and homogeneous Mo distribution in the doped sample. X-ray diffraction (XRD) revealed a structural transformation from a deformed orthorhombic phase in pristine Nb2O5 to a more crystalline pseudohexagonal phase in Mo-Nb2O5-500. Electrochemical analysis demonstrated a significant improvement in capacitive behavior, with Mo-Nb2O5-500 achieving a specific capacitance of 55.3 F/g at 5 mV/s, which is five times higher than the undoped sample. All electrodes exhibited stable cycling performance. These results highlight the synergistic role of Mo doping and calcination in enhancing the electrochemical properties of Nb2O5, offering a viable approach for developing high-performance pseudocapacitor electrodes.
Influence of Nb Dopant Concentration on the Structural Properties and Photocatalytic Performances of Hydrothermally Synthesized ZnO for Multi-Pollutant Degradation Quratul Aini; Carenina Isabel Suwono Putri; Rima Nurfitria; Istiara Rizqillah Hanifah
Greensusmater Vol. 3 No. 1 (2026)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/gsm.2026.01

Abstract

The development of effective photocatalysts for multi-pollutant wastewater remediation remains a significant environmental concern. In this study, Nb-doped ZnO photocatalysts with different Nb concentrations (0-6%) were synthesized using a hydrothermal process to systematically examine the influence of dopant concentration on materials characteristics and photocatalytic performance. According to X-ray diffraction analysis Nb incorporation preserved the hexagonal wurtzite ZnO structure with only slight lattice parameter changes, suggesting limited substitutional doping. Morphological observations showed that moderate Nb doping slightly enhanced particle structure and reduced agglomeration. The photocatalytic activity was evaluated through the degradation of ciprofloxacin (CIP) and methylene blue (MB) under UV irradiation, both in single and mixed pollutant systems. In single systems, the catalysts achieved high degradation efficiencies of up to 93.09% for CIP and 92.03% for MB after 120 min. In the mixed system, the efficiencies slightly decreased due to competitive interactions, reaching up to 87.57% (CIP) and 84.08% (MB). Kinetic analysis indicates pseudo-first-order behavior, with apparent rate constants (k) of approximately 0.0218 min<sup>−1</sup> (CIP) and 0.0199 min<sup>−1</sup> (MB) for the optimally doped Nb4-ZnO sample, which are comparable to those of pristine ZnO. The findings highlight the critical role of dopant concentration in tailoring structural and electronic properties, providing valuable insights into Nb-dopant optimization strategies for efficient multi-pollutant photocatalytic wastewater remediation.
A Novel Fiber Collection System for Rotary Force Spinning Method Dian Ahmad Hapidin; Elvina Ayu Ratnasari; Aan Priyanto; Khairurrijal Khairurrijal
Greensusmater Vol. 3 No. 1 (2026)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/gsm.2026.06

Abstract

Recent advancements in micro- to nano-scale fiber production, particularly through rotary force spinning (RFS), offer high production rates but face challenges in optimizing fiber collection efficiency. This study investigates the effect of spinneret angular speed on fiber collection performance of a novel RFS collector system. The collector system integrated zig-zag pole collectors with a rolling collector that seamlessly traverse between the poles for fiber assembly. This configuration enabled the produced fibers to be continuously assembled onto the rolling collector, thereby forming fibrous membranes directly during the spinning process. The collection performance was evaluated using polyvinylpyrrolidone (PVP) fibers fabricated at spinneret angular speeds ranging from 4000 to 11000 rpm. The results showed that the rolling collector captured up to 95.39% of the produced fibers at a high rotational speed of 11,000 rpm, whereas at lower rotational speed, most fibers were deposited onto the pole collectors, reaching 95.19% at 4000 rpm. These findings indicate that the proposed collector system effectively enhances fiber collection efficiency over a broad rotational speed range while enabling direct fibrous membrane formation in the RFS process.
Electrospun PAN/PVP/ZnO Nanofiber Membrane as a Photocatalyst for Methylene Blue Degradation under UV Irradiation Rut Rabekka Gultom; Istiara Rizqillah Hanifah; Rizky Aflaha; Hannah Faye M. Austria; T.M. Subrahmanya; Januar Widakdo; Aditya Rianjanu
Greensusmater Vol. 3 No. 1 (2026)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/gsm.2026.02

Abstract

Textile dye pollution remains a critical environmental concern, necessitating the development of efficient and recoverable photocatalysts for wastewater remediation. In this study, polyacrylonitrile/polyvinylpyrrolidone/zinc oxide (PAN/PVP/ZnO) nanofiber membranes were fabricated via electrospinning with varying ZnO loadings (0, 0.5, 1, and 2 mmol) and evaluated for the photocatalytic degradation of methylene blue (MB) under ultraviolet (UV) irradiation. Scanning electron microscopy (SEM) revealed continuous, bead-free nanofibers with mean diameters of 355–552 nm, and energy dispersive X-ray spectroscopy (EDS) confirmed systematic Zn incorporation up to 34.52 wt%. A comparative study demonstrated that heat treatment at 450 °C was essential for converting the Zn(NO<sub>3</sub>)<sub>2</sub> precursor into the photocatalytically active ZnO phase. X-ray diffraction (XRD) and Fourier-transform infrared spectroscopy (FTIR) confirmed the retention of the polymer matrix integrity. Among the tested formulations, PAN/PVP/ZnO-1 (1 mmol) exhibited the highest photocatalytic performance, achieving approximately 95% MB degradation within 180 min, with a pseudo-first-order rate constant of k = 0.0251 min<sup>−1</sup> (R<sup>2</sup> = 0.9926), approximately 9 times faster than the neat PAN/PVP membrane. Higher ZnO loading (2 mmol) resulted in reduced photocatalytic performance. These findings indicate that 1 mmol ZnO is the optimal loading for PAN/PVP nanofiber photocatalysts, offering a promising recoverable membrane system for photocatalytic dye removal from wastewater.
Electrospun ZnO Nanofiber Membranes for Photocatalytic Water Treatment: A Comparative Review of Fabrication Strategies Aditya Rianjanu; Eka Nurfani; Tarmizi Taher
Greensusmater Vol. 3 No. 1 (2026)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/gsm.2026.03

Abstract

Electrospun ZnO nanofiber membranes are promising candidates for photocatalytic water treatment, offering directional charge transport, high surface-to-volume ratio, and self-standing membrane architectures that enable straightforward catalyst retrieval and reuse, a critical advantage over dispersed semiconductor nanoparticle systems where post-treatment recovery remains a major bottleneck. However, the fabrication route fundamentally determines membrane morphology, mechanical integrity, retrievability, and photocatalytic performance. This review classifies electrospinning-based fabrication into three routes: the Ceramic Membrane Route (precursor/polymer blending followed by calcination), the Hierarchical Membrane Route (secondary ZnO growth on electrospun polymer scaffolds), and the Composite Membrane Route (direct electrospinning of pre-synthesized ZnO/polymer dispersions). The Ceramic Membrane Route yields high-crystallinity membranes with up to 100% pollutant degradation but poor mechanical integrity that hinders membrane retrieval. The Composite Membrane Route provides single-step fabrication with the best demonstrated reusability (10 cycles at 97–99% retention), 200-fold lower zinc leaching, and excellent mechanical robustness for repeated retrieval and deployment, positioning it as one of the more operationally mature options for near-term deployment. The Hierarchical Membrane Route delivers the highest surface area, the fastest degradation kinetics, and uniquely combines photocatalysis with membrane filtration in a single device, making it a particularly promising long-term direction once its multi-step processing is streamlined and continuous-flow scale-up is realized. This comparative framework guides the selection of fabrication strategy based on membrane retrievability, performance, and development-stage requirements.
Design and Optimization of CsPbI3 Perovskite Solar Cells Using SCAPS-1D Muhamad Kevin Ristiansyah; Bayu Prasetya; Mochammad Ghulam Isaq Khan; Muhammad Yasin Siregar; Abyan Abdillah Saoloan Panjaitan; Eri Widianto; Eka Nurfani
Greensusmater Vol. 3 No. 1 (2026)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/gsm.2026.04

Abstract

This study investigates the optimization of CsPbI<sub>3</sub>-based perovskite solar cells using SCAPS-1D simulation with a device structure of FTO/ZnO/CsPbI<sub>3</sub>/Spiro-OMeTAD/metal. Key parameters, including absorber thickness, defect density, acceptor concentration, and transport layer properties, were systematically analyzed. The results show that absorber thickness significantly affects device performance, with an optimal thickness of 1.6 μm yielding an efficiency of 17.66%. Optimization of defect density and acceptor concentration further enhances device performance. After overall optimization, the power conversion efficiency increases from 16.3% to 23.1%, with *V*<sub>oc</sub> improving from 1.19 V to 1.39 V, *J*<sub>sc</sub> from 18.33 to 20.5 mA/cm<sup>2</sup>, and FF from 75.2% to 87.4%. The improvement is supported by enhanced J–V characteristics and near-unity quantum efficiency over a wide wavelength range. These results demonstrate that parameter optimization plays a crucial role in achieving high-performance CsPbI<sub>3</sub> perovskite solar cells.
Effect of Composition and Morphology of Electrospun Polyacrylonitrile/Polyvinylpyrrolidone (PAN/PVP) Nanofibers on Adsorption of Methylene Blue and Congo Red Dyes Istiara Hanifah; Alex Triputra Lumban Tobing; Hanna Ronauli Permata Simamora; Anisa Fitri; Agita Phasa
Greensusmater Vol. 3 No. 1 (2026)
Publisher : Green and Sustainable Materials Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.62755/gsm.2026.05

Abstract

Synthetic dyes such as methylene blue (MB) and Congo red (CR) are persistent water pollutants requiring efficient removal. This study examines the effect of composition and morphology on the adsorption performance of electrospun polyacrylonitrile/polyvinylpyrrolidone (PAN/PVP) nanofiber membranes. PAN/PVP fibers with different PAN loadings (0.7–1.0 g, total polymer mass 1.3 g) were fabricated by electrospinning and subjected to hot-water soaking at 80 °C followed by thermal treatment at 200 °C. SEM and FTIR confirmed continuous nanofibrous networks containing both PAN and partially removed PVP, with only subtle morphological differences among compositions. Batch adsorption tests showed preferential uptake of MB over CR, with the highest MB capacity of 8.38 mg g<sup>−1</sup> obtained for the PAN/PVP-8 membrane and the highest CR capacity of 3.32 mg g<sup>−1</sup> obtained for the PAN/PVP-10 membrane, with only modest variation among the other ratios. Kinetic analysis revealed that MB and CR adsorption follow a pseudo-second-order model, indicating surface-controlled uptake and suggesting that further improvement will require targeted surface functionalization.

Page 3 of 3 | Total Record : 27

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