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Sorption Mechanism and Performance of Peat Soil Humin for Methylene Blue and p-Nitrophenol Sri Juari Santosa; Eko Sri Kunarti; Nurul Hidayat Aprilita; Beti Wulandari; Dhian Nuri Bawani
Indonesian Journal of Chemistry Vol 19, No 1 (2019)
Publisher : Universitas Gadjah Mada

The responsible mechanism and performance of peat soil humin for the sorption of methylene blue (MB) and p-nitrophenol (p-NP) have been investigated. Humin was obtained from peat soil of Siantan, West Kalimantan, Indonesia, after removing the content of humic and fulvic acids into a NaOH solution using the recommended procedure of International Humic Substances Society (IHSS). The obtained humin was then purified by rigorous stirring in a mixed solution of HCl 0.1 M and HF 0.3 M. Ash content in humin after the purification abruptly decreased from 36.84 to 1.26 wt.% indicating that minerals and other inorganic impurities were mostly removed. Phenolic –OH and carboxyl (–COOH) functional groups contributing to the acidity of humin were in the level of 3.44 and 2.10 mmol/g, respectively. At optimum medium pH of 6.20 for MB and 7.00 for p-NP, –COO– as the deprotonated product of –COOH was the most responsible active site in sorbing MB and p-NP through electrostatic interaction and hydrogen bonding, respectively. The homogeneity of –COO– as the active site for the sorption of MB and p-NP implied that the surface of humin sorbent was energetically uniform and thereby the sorption of both MB and p-NP followed better the Langmuir than the Freundlich isotherm model with sorption capacity of 0.19 and 0.26 mmol/g and sorption energy of 32.92 and 27.27 kJ/mol, respectively.

Development of a Simple Fe(II) Ion Colorimetric Sensor from the Immobilization of 1,10-Phenanthroline In Alginate/Pectin Film Nindya Tri Muliawati; Dwi Siswanta; Nurul Hidayat Aprilita
Indonesian Journal of Chemistry Vol 21, No 2 (2021)
Publisher : Universitas Gadjah Mada

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.22146/ijc.56759

An optical analytical sensor was proposed based on the complexation reactions of 1,10-phenanthroline derivative in aqueous solutions. This study aims to synthesize a metal ion sensor for detecting Fe(ll) ion from the immobilization of 1,10-phenanthroline compound in alginate/pectin film. This was carried out by characterizing the films using the Fourier-transform infrared spectrometry (FT-IR) and scanning electron microscope (SEM). The determination of the optimal condition for Fe(II) ion detection and validation of the parameters was conducted by measuring the absorbance of the films using a UV-Vis spectrophotometer. After the addition of Fe(II) ion, the color of the alginate/pectin-phenanthroline film changed from transparent yellow to orange-red, showing its potential as a visual colorimetric sensor for iron(II) ion. It was found that the optimum condition for Fe(II) ion sensing was at 513 nm after 2 min of detection at pH 2. The alginate/pectin-phenanthroline film had good linearity, precision, selectivity, and accuracy with a detection limit as low as 0.446 mg L–1, which was remarkable.

KAJIAN ANALISIS TERMAL KITIN-KITOSAN CANGKANG UDANG MENGGUNAKAN THERMOGRAVIMETRIC ANALYSIS DAN DIFFERENTIAL THERMAL ANALYSIS (TGA-DTA) Candra Purnawan; Nurul Hidayat Aprilita; Indriana Kartini; Eko Suguharto
Jurnal Sains dan Terapan Kimia Vol 2, No 2 (2008)
Publisher : Program Studi Kimia, Universitas Lambung Mangkurat

Telah dilakukan kajian analisis termal pada kitin-kitosan cangkang udang menggunakan thermogravimetric analysis dan differential thermal analysis (TGA-DTA). Kitosan dengan derajat deasetilasi (DD) bervariasi diperoleh dari proses deastilasi kitin dengan kondisi percobaan yang berbeda. Kitin dan kitosan dengan variasi DD tersebut dianalisis menggunakan TGA-DTA. Berdasarkan perbedaan termogram TGA-DTA kitin dan kitosan, menunjukkan bahwa kitosan lebih higroskopis daripada kitin dan memiliki gugus asetil yang lebih sedikit. Pada proses deasetilasi, kitin dimungkinkan terjadi degradasi rantai polimer dan pembentukan rantai polimer yang lebih panjang secara acak sehingga heterogenitas polimer kitosan lebih besar daripada kitin. Kata kunci: kitin-kitosan, analisis termal, termogram TGA/DTA

Heavy Metals Concentration in Muscle Tissue of Threatened Sharks (Rhizoprionodon acutus, Sphyrna lewini, and Squallus hemipinnis) from Binuangeun, Lebak Banten, Indonesia Suratno Suratno; Dwi Siswanta; Satriyo Krido Wahono; Nurul Hidayat Aprilita
Indonesian Journal of Chemistry Vol 22, No 4 (2022)
Publisher : Universitas Gadjah Mada

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.22146/ijc.72795

Metals accumulation in threatened sharks’ meat represents a global health issue. The objective of the current study was to measure the concentration of six metals (Li, Ti, Ni, Cd, As, and Pb) using ICP-MS in threatened sharks’ meat of Rhizoprionodon acutus, Squalus hemipinnis, and Sphyrna lewini from Binuangeun Fish Auction in Lebak, Banten, Indonesia. The results showed that the concentration of Ni, Li, Cd, and Pb was below the acceptable levels for food sources for human consumption, except for As concentration (more than 30 fold higher). This study showed high levels of Ti concentration in all threatened sharks' meat. Overall, this study shows that an accumulation of Ti in sharks' meat should be considered a risk to the health of seafood consumers.

Effect of Stirring Time on Sodium Silicate Synthesis From Mount Kelud Volcanic Ash Isna Nurhidayati; Endang Tri Wahyuni; Nurul Hidayat Aprilita; Sarwendah Ratnawati Hermanto
ALCHEMY:Journal of Chemistry Vol 9, No 2 (2021): ALCHEMY JOURNAL OF CHEMISTRY
Publisher : Department of Chemistry, Faculty of Science and Technology UIN Maulana Malik Ibrahim Malan

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.18860/al.v9i2.12600

This study performed the synthesis of sodium silicate from the volcanic ash of Mount Kelud with various stirring time in the sodium silicate synthesis process. Synthesis of sodium silicate was carried out using alkaline extraction at low temperature. This method is based on the solubility of silica under alkaline conditions and is proven to be more effective than the smelting method. The dissolution of silica contained in the volcanic ash of Mount Kelud was carried out using NaOH solution to form a Na2SiO3 solution. This process also studied the effect of stirring time on the amount of dissolved silica, with the stirring time of 0.5; 1; 1.5; 2; 2.5; 3 and 4 hours. The dissolved silica levels were tested using AAS. The amount of dissolved silica increased sharply with the longer length of stirring time, however for a stirring time of more than 2.5 hours, the dissolution was slow. The study revealed that the optimal result time was obtained from the stirring time of 2.5 hours with dissolved silica content of 19.82%. Keywords: volcanic ash, silica, sodium silicate, stirring time

ADSORPTION CHARACTERISTIC OF IRON ONTO POLY[EUGENOL-CO-(DIVINYL BENZENE)] FROM AQUEOUS SOLUTION Fitrilia Silvianti; Dwi Siswanta; Nurul Hidayat Aprilita; Agung Abadi Kiswandono
Jurnal Natural Volume 17, Number 2, September 2017
Publisher : Universitas Syiah Kuala

A study on the adsorption characteristic of Iron onto Poly[eugenol-co-(divinyl benzene)] (EDVB) from aqueous solution has been conducted. EDVB was produced and characterized by using FTIR spectroscopy. The adsorption was studied by a batch method by considering the factors affecting the adsorption such as initial metal ion concentration, adsorption selectivity, and mechanism of adsorption using a sequential desorption method. The adsorption of Iron onto EDVB followed a pseudo-2 order kinetics model with the rate constant of 0,144 L2 mmol-1 min-1. The adsorption isotherm was studied with Tempkin, Langmuir and Freundlich models. The adsorption capacity (Qmax) obtained by Langmuir isotherms was 250mg.L-1 while the equilibrium value was 0.8 Lmg-1. A competitive adsorption study showed that EDVB is adsorbed selectively towards Iron rather than Chromium, Coppers and Cadmium ions. The interaction type of Iron onto EDVB was determined by a sequential desorption.Keywords: Polyeugenol; divinyl benzene (DVB); adsorption; Iron; FeReferencesAbasi, C. Y.; Abia, A.A.; Igwe, J.C. Adsorption of Iron (III), Lead (II) and Cadmium (II) Ions by Unmodified Raphia Palm (Raphia hookeri) Fruit Endocarp. Environ. Res. 2011, 5 (3), 104-113, ISSN: 1994-5396, Medwell Journals. DOI: 10.3923/erj.2011.104.113Baes, F. C.; Mesmer, R. E. The Hydrolisis of Cations; John Wiley: New York, 1976Bakatula, E.N.; Cukrowska, E.M.; Weiersbye, L.; Mihali-Cozmuta, L.;Tutu, H. Removal of toxic elements from aqueous solution using bentonite modified with L-histidine. Water Sci. Technol.2014, 70 (12),2022-2030, DOI: 10.2166/wst.2014.450Bhattacharyya, K.G.; Gupta, S.S. Adsorption of Fe(III) from Water by Natural and Acid Activated Clays: Studies on equilibrium isotherm, kinetics and thermodynamics of interactions. Adsorption. 2006, 12 (3), 185-204,DOI : 10.1007/s10450-006-0145-0Carmona, M..; Lucas, A.D.; Valverde, J.L.; Velasco, B.; Rodriguez, J.F. Combined adsorption and ion exchange equilibrium of phenol on Amberlite IRA-420.Chem. Eng. J.2006, 117, 155-160, Doi : 10.1016/j.cej.2005.12.013Debnath, S.; Ghosh, U.C. Kinetics, isotherm and thermodynamics for Cr(III) and Cr(VI) adsorption from aqueous solutions by crystalline hydrous titanium oxide. J. Chem. Thermodin. 2008, 40: 67-77, DOI: 10.1016/j.jct.2007.05.014Djunaidi, M.C.; Jumina; Siswanta, D.; Ulbricht, M. Selective Transport of Fe(III) Using Polyeugenol as Functional Polymer with Ionic Imprinted Polymer Membrane Method. Asian J. Chem. 2015, 27 (12): 4553-4562, DOI : 10.14233/ajchem.2015.19228Febriasari, A.; Siswanta, D.; Kiswandono, A.A.; Aprilita, N.H. Evaluation of Phenol Transport Using Polymer Inclusion Membrane (PIM) with Polyeugenol as a Carrier. Jurnal Rekayasa Kimia dan Lingkungan. 2016, Vol. 11, No. 2, 99-106, DOI: 10.23955/rkl.v11i2.5112Foldesova, M.; Dillinger, P.; Luckac, P. Sorption and Desorption of Fe(III) on Natural and chemically modified zeolite. J. Radioanal. Nucl. Chem. 1999, Vol. 242, No. 1 (1999), 227-230, DOI: 10.1007/BF02345926Gupta, V.K.;Sharma, S. Removal of cadmium and zinc from aqueous solutions using mud.Environ. Sci. Technol. 2002, 36: 3612-3617, DOI: 10.1021/es020010vHandayani, D.S. Sintesis kopoli(eugenol-DVB) sulfonat dari Eugenol Komponen Utama Minyak Cengkeh Szygium aromaticum (Synthesis of copoly(eugenol-DVB) sulfonic from main components of eugenol clove oil Szygium aromaticum). Biopharmacy Journal of Pharmacological and Biological Sciences. 2004, 2 (2): 53-57 ISSN: 1693-2242. url : https://eprints.uns.ac.id/id/eprint/856Harimu, L.; Matsjeh, S.; Siswanta, D.; Santosa, S.J. Synthesis of Polyeugenyl Oxyacetic Acid as Carrier to Separate Heavy Metal Ion Fe(III), Cr(III), Cu(II), Ni(II), Co(II), and Pb(II) that Using Solvent Extraction Mehod. Indo. J. Chem. 2009, 9 (2): 261-266.Ho, Y.S.; McKay, G. Pseudo-second Order Model for Sorption Processes. Process. Biochem. 1999, 34, 451-465, DOI: 10.1016/S0032-9592(98)00112-5Ho, Y.S.; McKay, G.; Wase, D.A.J.;Forster, C.F. Study of Sorption Divalent Metal Ions on to Peat. Adsorpt. Sci. Technol. 2000, 18: 639-650. DOI : 10.1260/0263617001493693Indah, S.; Helard, D.;Sasmita, A. Utilization of maize husk (Zea mays L.) as low-cost adsorbent in removal of iron from aqueous solution. Water Sci. Technol. 2016, 73 (12), 2929-2935, DOI: 10.2166/wst.2016.154Kiswandono, A.A.; Siswanta, D.; Aprilita, N.H.; Santosa, S.J. Transport of Phenol through inclusion polymer membrane (PIM) using copoly(Eugenol-DVB) as membrane carries. Indo .J. Chem. 2012, 12 (2): 105-112. Doi : 10.22146/ijc.667Kousalya, N.; Gandhi, M.R.; Sundaram, C.S.; Meenakshi, S. Synthesis of nano-hydroxyapatite chitin/chitosan hybrid bio-composites for the removal of Fe(III).Carbohyd. Polym. 2010, 82: 594-599, DOI:10.1016/j.carbpol.2010.05.013Kumar, K.V.; Porkodi, K.;Rocha, F. Langmuir-Hinshelwood kinetics – A theoretical study, Catalysis Communications. 2008, 9: 82-84, DOI:10.1016/j.catcom.2007.05.019Masel, R.I. Principles Adsorption and Reaction on Solid Surface; John Wiley Sons: Canada, 1996Moore, J. W.; Pearson, R.G. Kinetics and Mechanism Third Edition; John Wiley Sons: Canada, 1981.Ngah, W.S.W.; Ghani, S.A.; Kamari, A. Adsorption Behaviour of Fe(II) and Fe(III) Ions in Aqueous Solution on Chitosan and Cross-linked Chitosan Beads. Bioresource. Technol. 2005, 96: 443-450. DOI:10.1016/j.biortech.2004.05.022Rahim, E.A.; Sanda, F.; Masuda, T. Synthesis and Properties of Novel Eugenol-Based Polymers. Polymer Bulletin. 2004, Vol. 5, 93-100, DOI: 10.1007/s00289-004-0272-2Samarghandi, M.R.; Hadi. M.; Moayedi, M.; Askari, F.B. 2009. Two Parameter Isotherms of Methyl Orange Sorption by Pinecone Derived Activated Carbon. Iran. J. Environ. Health Sci. Eng., 6 (4): 285-294.Setyowati, L. 1998. Pengaruh Penambahan Divinil Benzena (DVB) pada Kopolimerisasi Kationik Poli[eugenol-co-(divinil benzena)] dan Sifat Pertukaran Kation Kopoligaramnya (The Effect of divinylbenzene (DVB) Addition to Eugenol-DVB Cationic Copolymerization and Its Use As Cation-Exchanger), Thesis, Faculty of Mathematics and Natural Sciences, Universitas Gadjah Mada, Yogyakarta, Indonesia.Shi, T.; Jia, S.; Chen, Y.; Wen, Y.; Du, C.; Guo, H.; Wang, Z. Adsorption of Pb(II), Cr(III), Cu(II), Cd(II) and Ni(II) onto a vanadium mine tailing from aqueous solution. J. Hazard. Mater. 2009, 169: 838-846, DOI: 10.1016/j.jhazmat.2009.04.020Sun, S.;Wang, A. Adsorption Kinetics of Cu(II) Ions Using N,O-Carboxymethyl-Chitosan. J. Hazard. Mater. 2006, B131: 103-111, DOI: 10.1016/j.jhazmat.2005.09.012Sun, S.; Wang, L.;Wang, A. Adsorption Properties of Crosslinked Carboxymethyl-chitosan Resin With Pb(II) as Template Ions. J. Hazard. Mater. 2006, B136: 930-937, DOI: 10.1016/j.jhazmat.2006.01.033Uzun, I.; Guzel, F. Adsorption of Some Heavy Metal Ions from Aqueous Solution by Activated Carbon and Comparison of Percent Adsorption Result of Activated Carbon with those of Some Other Adsorbents. Turk. J. Chem. 2000, 24: 291-297.Zou, X.; Pan, J.; Ou, H.; Wang, X.;Guan, W.; Li, C.; Yan, Y.; Duan, Y. Adsorptive removal of Cr(III) and Fe(III) from aqueous solution by chitosan/attapulgite composites: Equilibrium, thermodynamics and kinetics. Chem. Eng. J. 2011, 167: 112-121, DOI: 10.1016/j.cej.2010.12.009

Advanced Oxidation Processes of Amoxicillin Based on Visible Light Active Nitrogen-Doped TiO2 Photocatalyst Kusuma Putri Suwondo; Nurul Hidayat Aprilita; Endang Tri Wahyuni
Indonesian Journal of Chemistry Vol 23, No 2 (2023)
Publisher : Universitas Gadjah Mada

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.22146/ijc.81387

Environmental consequences during the COVID-19 pandemic have attracted attention due to the excessive use of antibiotics which lead to the release of the drug's residue, such as amoxicillin (AMX), into the environment. In this work, an advanced oxidation process based on a visible, active N-doped TiO2 photocatalyst was carried out to eliminate AMX. Nitrogen with different initial doping concentrations (15, 30, 45% w/w) was doped into TiO2 by the sol-gel method. The characterization technique such as XRD, FTIR, UV-SRS, and SEM-EDX revealed that nitrogen with 30% doping concentration improved the TiO2 response in the visible region, attributed to the lower band gap energy (2.97 eV). In the photodegradation processes, the TiO2-N (30%) photocatalyst possessed higher AMX degradation than undoped TiO2 for both UV and visible light irradiation. In an aqueous solution, the degradation percentage of AMX by TiO2-N (30%) was 68.5 and 84.12%, while the degradation percentage of AMX by TiO2 was 38.7 and 78.01% under visible and UV light, respectively.

Development of Methylmercury Analysis by Ultra-High Performance Liquid Chromatography Coupled with ICP-MS and Its Application on Sharks’ Meat Measurement Suratno Suratno; Satriyo Krido Wahono; Dwi Siswanta; Nurul Hidayat Aprilita
Indonesian Journal of Chemistry Vol 23, No 3 (2023)
Publisher : Universitas Gadjah Mada

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.22146/ijc.82512

This study analyzed MeHg in a fast, simple, low-waste, and accurate by using ultra-high liquid chromatography coupled with inductively coupled plasma mass spectrometry. Simple preparation by liquid extraction with sonication at room temperature was effective extract MeHg from Certified Reference Material (CRM) and shark meat samples. Effective MeHg separation was achieved in less than 300 s using a C18 Hypersil Gold analytical column with a mobile gradient phase of 0.5% (w/v) L-cysteine in 2% (v/v) HNO3 and 100% methanol. The MeHg was extracted from 100 mg of shark meat using 1 mL of 0.5% (w/v) L-cysteine in 2% (v/v) HNO3 and sonicated for 30 min. Analysis of certified reference material (DORM-4) showed values between the experimental and certified values. The observed limit of detection and quantification MeHg were 0.86 and 2.85 pg/L, respectively. This method was applied to measure MeHg in shark meat from Binuangeun areas. The MeHg concentration in Rhizoprionodon acutus was 0.22–0.63 mg/kg wet weight (w.w.), Squalus hemipinis 0.68–1.14 mg/kg w.w., and 0.29–1.22 mg/kg w.w. for Sphyrna lewini. This study provides a quick and easy method to evaluate MeHg in shark meat or other seafood products and applies to many samples in a single assay.

THE INFLUENCE OF OXALIC AND MALONIC ACIDS ON THE DEGREE OF Cu(II) PHOTOREDUCTION CATALYZED BY TIO2 (Pengaruh Asam Oksalat dnn Malonst terhadap Derajad Fotoreduksi ion Cu(II) yang Terkatalisis oleh TiO2) Endang Tri Wahyuni; Nurul Hidayat Aprilita; An Nissa F. Hayu; Siti Nurhayati
Jurnal Manusia dan Lingkungan Vol 15, No 1 (2008): Maret
Publisher : Pusat Studi Lingkungan Hidup Universitas Gadjah Mada

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.22146/jml.18674

The influence of oxalic and malonic acids on the effectiveness of Cu(ll) photoreduction catalyzed by TiO, has been studied. Photoreduction was carried out by a batch system in a closed reactor equipped by UV lamp. The results of the research show that the addition of TiO, photocatalyst can enhance Cu(ll) photocatalytic reduction, which may be initiated and/or accompanied by adsorption of Cu(ll) ion on the TiO, surface. The presence of both oxalic and malonic acids can improve of the Cu(ll) photoreduction, and the improvement is observed as the acid concentrations increase. It is also found that the effect of malonic acid in gaining Cu(ll) photoreduction is stronger than oxalic is, which are from around 20% into about 55% and that of into aroun d 35%, respectively. The roles of the acids on the enhancement of the photoreduction are OH radical attachment and electron donation.

ADSORPTION CHARACTERISTIC OF IRON ONTO POLY[EUGENOL-CO-(DIVINYL BENZENE)] FROM AQUEOUS SOLUTION Fitrilia Silvianti; Dwi Siswanta; Nurul Hidayat Aprilita; Agung Abadi Kiswandono
Jurnal Natural Volume 17, Number 2, September 2017
Publisher : Universitas Syiah Kuala

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.24815/jn.v17i2.8076

A study on the adsorption characteristic of Iron onto Poly[eugenol-co-(divinyl benzene)] (EDVB) from aqueous solution has been conducted. EDVB was produced and characterized by using FTIR spectroscopy. The adsorption was studied by a batch method by considering the factors affecting the adsorption such as initial metal ion concentration, adsorption selectivity, and mechanism of adsorption using a sequential desorption method. The adsorption of Iron onto EDVB followed a pseudo-2 order kinetics model with the rate constant of 0,144 L2 mmol-1 min-1. The adsorption isotherm was studied with Tempkin, Langmuir and Freundlich models. The adsorption capacity (Qmax) obtained by Langmuir isotherms was 250mg.L-1 while the equilibrium value was 0.8 Lmg-1. A competitive adsorption study showed that EDVB is adsorbed selectively towards Iron rather than Chromium, Coppers and Cadmium ions. The interaction type of Iron onto EDVB was determined by a sequential desorption.Keywords: Polyeugenol; divinyl benzene (DVB); adsorption; Iron; FeReferencesAbasi, C. Y.; Abia, A.A.; Igwe, J.C. Adsorption of Iron (III), Lead (II) and Cadmium (II) Ions by Unmodified Raphia Palm (Raphia hookeri) Fruit Endocarp. Environ. Res. 2011, 5 (3), 104-113, ISSN: 1994-5396, Medwell Journals. DOI: 10.3923/erj.2011.104.113Baes, F. C.; Mesmer, R. E. The Hydrolisis of Cations; John Wiley: New York, 1976Bakatula, E.N.; Cukrowska, E.M.; Weiersbye, L.; Mihali-Cozmuta, L.;Tutu, H. Removal of toxic elements from aqueous solution using bentonite modified with L-histidine. Water Sci. Technol.2014, 70 (12),2022-2030, DOI: 10.2166/wst.2014.450Bhattacharyya, K.G.; Gupta, S.S. Adsorption of Fe(III) from Water by Natural and Acid Activated Clays: Studies on equilibrium isotherm, kinetics and thermodynamics of interactions. Adsorption. 2006, 12 (3), 185-204,DOI : 10.1007/s10450-006-0145-0Carmona, M..; Lucas, A.D.; Valverde, J.L.; Velasco, B.; Rodriguez, J.F. Combined adsorption and ion exchange equilibrium of phenol on Amberlite IRA-420.Chem. Eng. J.2006, 117, 155-160, Doi : 10.1016/j.cej.2005.12.013Debnath, S.; Ghosh, U.C. Kinetics, isotherm and thermodynamics for Cr(III) and Cr(VI) adsorption from aqueous solutions by crystalline hydrous titanium oxide. J. Chem. Thermodin. 2008, 40: 67-77, DOI: 10.1016/j.jct.2007.05.014Djunaidi, M.C.; Jumina; Siswanta, D.; Ulbricht, M. Selective Transport of Fe(III) Using Polyeugenol as Functional Polymer with Ionic Imprinted Polymer Membrane Method. Asian J. Chem. 2015, 27 (12): 4553-4562, DOI : 10.14233/ajchem.2015.19228Febriasari, A.; Siswanta, D.; Kiswandono, A.A.; Aprilita, N.H. Evaluation of Phenol Transport Using Polymer Inclusion Membrane (PIM) with Polyeugenol as a Carrier. Jurnal Rekayasa Kimia dan Lingkungan. 2016, Vol. 11, No. 2, 99-106, DOI: 10.23955/rkl.v11i2.5112Foldesova, M.; Dillinger, P.; Luckac, P. Sorption and Desorption of Fe(III) on Natural and chemically modified zeolite. J. Radioanal. Nucl. Chem. 1999, Vol. 242, No. 1 (1999), 227-230, DOI: 10.1007/BF02345926Gupta, V.K.;Sharma, S. Removal of cadmium and zinc from aqueous solutions using mud.Environ. Sci. Technol. 2002, 36: 3612-3617, DOI: 10.1021/es020010vHandayani, D.S. Sintesis kopoli(eugenol-DVB) sulfonat dari Eugenol Komponen Utama Minyak Cengkeh Szygium aromaticum (Synthesis of copoly(eugenol-DVB) sulfonic from main components of eugenol clove oil Szygium aromaticum). Biopharmacy Journal of Pharmacological and Biological Sciences. 2004, 2 (2): 53-57 ISSN: 1693-2242. url : https://eprints.uns.ac.id/id/eprint/856Harimu, L.; Matsjeh, S.; Siswanta, D.; Santosa, S.J. Synthesis of Polyeugenyl Oxyacetic Acid as Carrier to Separate Heavy Metal Ion Fe(III), Cr(III), Cu(II), Ni(II), Co(II), and Pb(II) that Using Solvent Extraction Mehod. Indo. J. Chem. 2009, 9 (2): 261-266.Ho, Y.S.; McKay, G. Pseudo-second Order Model for Sorption Processes. Process. Biochem. 1999, 34, 451-465, DOI: 10.1016/S0032-9592(98)00112-5Ho, Y.S.; McKay, G.; Wase, D.A.J.;Forster, C.F. Study of Sorption Divalent Metal Ions on to Peat. Adsorpt. Sci. Technol. 2000, 18: 639-650. DOI : 10.1260/0263617001493693Indah, S.; Helard, D.;Sasmita, A. Utilization of maize husk (Zea mays L.) as low-cost adsorbent in removal of iron from aqueous solution. Water Sci. Technol. 2016, 73 (12), 2929-2935, DOI: 10.2166/wst.2016.154Kiswandono, A.A.; Siswanta, D.; Aprilita, N.H.; Santosa, S.J. Transport of Phenol through inclusion polymer membrane (PIM) using copoly(Eugenol-DVB) as membrane carries. Indo .J. Chem. 2012, 12 (2): 105-112. Doi : 10.22146/ijc.667Kousalya, N.; Gandhi, M.R.; Sundaram, C.S.; Meenakshi, S. Synthesis of nano-hydroxyapatite chitin/chitosan hybrid bio-composites for the removal of Fe(III).Carbohyd. Polym. 2010, 82: 594-599, DOI:10.1016/j.carbpol.2010.05.013Kumar, K.V.; Porkodi, K.;Rocha, F. Langmuir-Hinshelwood kinetics – A theoretical study, Catalysis Communications. 2008, 9: 82-84, DOI:10.1016/j.catcom.2007.05.019Masel, R.I. Principles Adsorption and Reaction on Solid Surface; John Wiley Sons: Canada, 1996Moore, J. W.; Pearson, R.G. Kinetics and Mechanism Third Edition; John Wiley Sons: Canada, 1981.Ngah, W.S.W.; Ghani, S.A.; Kamari, A. Adsorption Behaviour of Fe(II) and Fe(III) Ions in Aqueous Solution on Chitosan and Cross-linked Chitosan Beads. Bioresource. Technol. 2005, 96: 443-450. DOI:10.1016/j.biortech.2004.05.022Rahim, E.A.; Sanda, F.; Masuda, T. Synthesis and Properties of Novel Eugenol-Based Polymers. Polymer Bulletin. 2004, Vol. 5, 93-100, DOI: 10.1007/s00289-004-0272-2Samarghandi, M.R.; Hadi. M.; Moayedi, M.; Askari, F.B. 2009. Two Parameter Isotherms of Methyl Orange Sorption by Pinecone Derived Activated Carbon. Iran. J. Environ. Health Sci. Eng., 6 (4): 285-294.Setyowati, L. 1998. Pengaruh Penambahan Divinil Benzena (DVB) pada Kopolimerisasi Kationik Poli[eugenol-co-(divinil benzena)] dan Sifat Pertukaran Kation Kopoligaramnya (The Effect of divinylbenzene (DVB) Addition to Eugenol-DVB Cationic Copolymerization and Its Use As Cation-Exchanger), Thesis, Faculty of Mathematics and Natural Sciences, Universitas Gadjah Mada, Yogyakarta, Indonesia.Shi, T.; Jia, S.; Chen, Y.; Wen, Y.; Du, C.; Guo, H.; Wang, Z. Adsorption of Pb(II), Cr(III), Cu(II), Cd(II) and Ni(II) onto a vanadium mine tailing from aqueous solution. J. Hazard. Mater. 2009, 169: 838-846, DOI: 10.1016/j.jhazmat.2009.04.020Sun, S.;Wang, A. Adsorption Kinetics of Cu(II) Ions Using N,O-Carboxymethyl-Chitosan. J. Hazard. 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