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Himawan Tri Bayu Murti Petrus
Departemen Teknik Kimia, Fakultas Teknik, Universitas Gadjah Mada, Jl Grafika No. 2 Kampus UGM, Yogyakarta, 55281
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Journal : Bulletin of Chemical Reaction Engineering

 1 
Bimetallic Ni-Fe Supported by Gadolinium Doped Ceria (GDC) Catalyst for CO2 Methanation Kristiani, Anis; Takeishi, Kaoru; Jenie, Siti Nurul Aisyiyah; Petrus, Himawan Tri Bayu Murti
Bulletin of Chemical Reaction Engineering & Catalysis 2024: BCREC Volume 19 Issue 1 Year 2024 (April 2024)
Publisher : Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.9767/bcrec.20108

Abstract

CO2 conversion into fuels and high value-added chemical feedstocks, such as methane, has gained novel interest as a crucial process for further manufacturing multi-carbon products. Methane, CH4, becomes a promising alternative for environmental and energy supply issues. Nickel-based catalysts were found to be very active and selective for CH4 production. The use of promoter and support material to develop high activity, high selectivity, and durable catalysts for CO2 methanation at low temperature is a challenge. Gadolinium-Doped Ceria (GDC) has been known as material for Solid Oxide Fuel Cell (SOFC) and Solid Oxide Electrolysis Cell (SOEC) due to higher ionic conductivity and lower operating temperatures. However, few researches have been done regarding to CO2 methanation over GDC as catalyst support so far. In this present work, CO2 methanation was investigated over bimetallic Ni-Fe catalyst supported by GDC. The results showed that CH4 production rate by using Ni-Fe/GDC catalyst was higher than that of GDC at all reaction temperatures carried on. Ni-Fe/GDC showed remarkable CH4 production rate as of 17.73 mmol.gcat−1.h−1 at 280 °C. No catalytic activity was produced by GDC catalyst only. The highest CO2 conversion (46.50%) was observed at 280 °C, with almost 100% selectivity to CH4. The turnover frequency (TOF) value of Ni-Fe/GDC (4529.32 h−1) was the highest than that of Ni and common CO2 methanation catalyst, Ni/Al2O3 catalysts at 280 °C, further displaying the outstanding low-temperature catalytic activity. Copyright © 2024 by Authors, Published by BCREC Publishing Group. This is an open access article under the CC BY-SA License (https://creativecommons.org/licenses/by-sa/4.0).
Co-Authors Achmad Roesyadi Adha Priyawan, Adha Adiatama, Aufa Rai Adythia, Dicky Marsa Agus Haerudin Agus Prasetya Agus Prasetya Ahmad Tawfiequrrahman Yuliansyah Akbar Yulandra Althea Farina Atmaja, Althea Farina Anastasia Prima Kristijarti Andi Nurfaadilah Ulfah Angelia, Annasthasya Milleni Anis Kristiani, Anis Aprilianto, Doni Riski Ardyanto Wijaya Arham, La Ode Arifudin Idrus Arini Nur Utami Asih, Yekti Aulia Pertiwi Tri Yuda Bahri, Elsha Pamida Bangun, Aya Shika Bratakusuma, Danu Bratakusuma, Danu BUDI SETIADI DARYONO Christopher Mario Hananto Chusnul Khotimah Cipta Panghegar Supriadi D Bratakusuma Dagus Resmana Djuanda Danu Bratakusuma Danu Bratakusuma Dea Anisa Ayu Besari Devi, Fatma Putrinta Dewi Purnama Sari Dewi Purnama Sari Dewi, Jilda Sofiana Dwi Umi Siswanti Dwi Wiji Lestari Edward Yonathan Natapraja Eko Agus Suyono Elsha Pamida Bahri Fahrurozi, Mohammad Fajar Nurjaman Fajar Nurjaman Fathan Bahfie Febry Yulindra Abdi Saputra Federick Dwi Putra Federick Dwi Putra Felisha Hapsari Tanujaya Felisha Hapsari Tanujaya Felix Arie Setiawan Ferian Anggara Fika Rofiek Mufakhir Fika Rofiek Mufakhir Fika Rofiek Mufakir Fika Rofiek Mufakir Fika Rofieq Mufakhir Franky Michael Hamonangan Siagian Gelar Panji Gemilar Gelar Panji Gemilar Gemilar, Gelar Panji Gyan Prameswara Hafid Zul Hakim Halomoan Siagian Harta Haryadi, Harta Hazmi, Fariz Al Heimbach, Ivano Hendrik Setiawan Hendrik Setiawan, Hendrik Himmah Sekar Eka Ayu Agustina Hotden Manurung Hotden Manurung I Gde Sukadana I Made Bendiyasa I Wayan Christ Widhi Herman Tangkas I Wayan Warmada Iga Trisnawati Iga Trisnawati Indra Perdana Indra Perdana Indra Perdana Indra Perdana Istihanah Nurul Eskani Ivanna Crecentia Narulita Simanungkalit Jayawarsa, A.A. Ketut Jonas Kristanto Joni Setiawan Kevin Cleary Wanta Kinanti, Divita Hayyu Kristanto, Jonas Kurniawansyah, Firman Laksono Trisnantoro Marizka Aviana Permatasari Mita Kusumaningrum, Mita Mufakhir, Fika Rofiek Mufakhir, Fika Rofieq Muhammad Miftahur Rahman Mustika, Pra Cipta Buana Wahyu Nadya Fardani, Nadya Nasution, Yogi Tri Putra Natalia, Priskila Patria, Aulia Agus Perbawati, Esti Kukuh Poernomo, Venny Pratiwi, Fadiah Putra, Agik Dwika Putra, Ilham Satria Raditya Radinda Bian Zaqina, Radinda Bian Rahman, Muhammad Irfan Rahman, Muhammad Miftahur Ramadhany, Putri Ratna Frida Susanti Rika Ernawati Riyadi, Delfimelinda Nurul RR. Ella Evrita Hestiandari Salafudin Salafudin, Salafudin Shinta Virdhian Shinta Virdhian shinta virdhian, shinta Siagian, Franky Michael Hamonangan Simanungkalit, Ivanna Crecentia Narulita Siti Nurul Aisyiyah Jenie, Siti Nurul Aisyiyah Slamet Sumardi Slamet Sumardi Slamet Sumardi, Slamet Soesaptri Oediyani Stephen Lim Stevanus Adi Darma Sujoto, Vincent Sutresno Hadi Supit, Jance Mudjani Suprabanindya, Caecilia Tridjata Supriadi , Cipta Panghegar Supriyatna, Yayat Iman Surianti Surianti Suryanaga, Chandra Edward Suryanaga, Edward Chandra Sutijan Sutijan Sutijan Sutijan Sutopo, Ulung Syamsumin Syamsumin, Syamsumin Takeishi, Kaoru Tampubolon, Aron Pangihutan Christian Tangkas, I Wayan Christ Widhi Herman Taufik Hery Purwanto Timotius, Daniel Trisnawati, Iga Ulfah , Andi Nurfaadilah Ulin Herlina Ulung Sutopo Utama, Andhika Putera Utomo, Dimas Bagus Galih Vincent Sutresno Hadi Sujoto Wahyu Rachmi pusparini Wahyu Yun Santoso Wibowo, Decka Pynka Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widi Astuti Widya Rosita Wijaya, Ardyanto Wiratni Wiratni Wiratni Wiratni, Wiratni Y Iskandar Yogi Tri Putra Nasution Yuda, Aulia Pertiwi Tri Yuni Kusumastuti, Yuni Yuniati, Mutia Dewi Yusuf Iskandar