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All Journal VALENSI CAKRA KIMIA (Indonesian E-Journal of Applied Chemistry) Jurnal Kimia (Journal of Chemistry) CHEMISTRY PROGRESS International Journal of Science and Engineering (IJSE) Jurnal Penelitian Sains (JPS) Jurnal Kedokteran Brawijaya Jurnal Matematika & Sains Bulletin of Chemical Reaction Engineering & Catalysis The Journal of Pure and Applied Chemistry Research AGRIVITA, Journal of Agricultural Science Jurnal Penelitian Sains (JPS) IJFAC (Indonesian Journal of Fundamental and Applied Chemistry) JPSriwijaya Indonesian Journal of Chemical Science Science and Technology Indonesia Jurnal Penelitian Sains Indonesian Journal of Chemistry Communications in Science and Technology IJEMS (Indonesian Journal of Environmental Management and Sustainability) Riau Journal of Empowerment Molekul: Jurnal Ilmiah Kimia Sains dan Matematika SRIWIJAYA JOURNAL OF ENVIRONMENT Makara Journal of Science Makara Journal of Technology Aceh International Journal of Science and Technology Karunia: Jurnal Hasil Pengabdian Masyarakat Indonesia Bulletin of Chemical Reaction Engineering & Catalysis Indonesian Journal of Material Research Bumi: Jurnal Hasil Kegiatan Sosialisasi Pengabdian Kepada Masyarakat
Aldes Lesbani
Universitas Sriwijaya
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Journal : Bulletin of Chemical Reaction Engineering

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Green-Modified Ni/Al LDH with Camellia sinensis Bioactives: A Sustainable Strategy for Ceftriaxone Removal Amri, Amri; Fithri, Najma Annuria; Said, Muhammad; Lesbani, Aldes
Bulletin of Chemical Reaction Engineering & Catalysis 2025: Just Accepted Manuscript and Article In Press 2025
Publisher : Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.9767/bcrec.20513

Abstract

Ceftriaxone (CEF) is a β-lactam antibiotic widely used in the medical field to treat various bacterial infections in both humans and animals. The high usage of CEF has the potential to cause environmental pollution and antimicrobial resistance, necessitating effective treatment methods. In this study, the adsorption method is proposed using Ni/Al layered double hydroxide (LDH) and Camellia sinensis extract-modified material (Ni/Al-CSe) as a sustainable bio-modification approach. The results show the optimal adsorption pH for Ni/Al LDH is 3 and for Ni/Al-CSe is 5, with the adsorption isotherms following the Freundlich model and the kinetics conforming to pseudo-first order (PFO). The maximum adsorption capacity (Qm) significantly increased from 28.818 mg/g (Ni/Al LDH) to 111.111 mg/g (Ni/Al-CSe). Thermodynamic analysis revealed that adsorption on both materials proceeds spontaneously, while the consistently more negative ΔG values and predominantly exothermic behavior of Ni/Al-CSe confirm its superior thermodynamic favorability associated with more specific surface interactions. Regeneration tests up to four cycles showed that Ni/Al-CSe was more stable than Ni/Al LDH. Overall, modifying Ni/Al LDH with Camellia sinensis extract was proven to enhance adsorption capacity, spontaneity, and stability, providing an effective and environmentally friendly solution for antibiotic treatment.
Co-Authors A. Agnes Abi Sueb Abriyanto, Danang Addy Rachmat Adi Saputra Adi Saputra Adi Saputra Adi Saputra Afifah Rahma Dian Ahmad Fatoni Ahmad Fatoni Alfan Wijaya Alfan Wijaya Alfan Wijaya Amiruddin Supu Amri Amri Amri Andi Wijaya Andreas, Roy Andriani Azora Andriani Azora Anggraini, Ana Arini Fousty Badri Arini Fousty Badri Arison Musri Arison Musri Arsyad, Fitri Suryani Aslihati Aslihati Aslihayati Aslihayati Azhar Kholiq Badri, Arini Fousty Bakri Rio Rahayu Bakri Rio Rahayu Benyamin Lakitan Dedi Rohendi Dedi Setiabudidaya Desnelli Desnelli Dian Monariqsa Dian Monariqsa Didi Jasantri Dormian A N Haloho Dormian A N Haloho Eiffel Ostan Jeski Gultom Elfita Elfita . Elfita Elfita Eliza . Eliza Eliza Eliza Eliza Ema Veronika Turnip Endri Junaidi Eriza Sativa Erviana, Desti Fahma Riyanti Fatmawati Fatmawati Ferlinahayati Ferlinahayati Fitri Suryani Arsyad Fitri, Erni Salasia Fitriliana Fitriliana Hanifah, Yulizah Haris Kriswantoro Hermansyah Hermansyah Hermansyah Hermansyah Hesti A. Harahap Hesti A. Harahap, Hesti Hidayatullah, Muhammad Hilda Zulkifli Hilda Zulkifli Hilda Zulkifli Hiroshi Nishihara Hitoshi Kondo Idha Royani Intan Permata Sari Irfannuddin Irfannuddin Jasantri, Didi Jefri Jefri Jeri Ramadhan Juleanti, Novie Kiki Anggraini Kiki Anggraini Kiki Anggraini, Kiki Komis Krisna Murti Laila Hanum Leni Sinaga Lestari Simanjuntak Lestari Simanjuntak Liasari, Beta Riana Lingga, Fitra Wahyuni Lora Vitanesa Lucyanti . Lucyanti Lucyanti Lusi Teresia Mardianto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto Mardiyanto, Marieska Verawaty Mariska Verawaty Melantina Melan Oktriyanti Melwita, Elda Menik Setyowati Mikha Meilinda Christina Miksusanti Miksusanti Muhammad Imron MUHAMMAD SAID Muhammad Said Muhammad Said Muhammad Said Najma Annuria Fithri Najma Annuria Fithri Najma Annuria Fithri Najma Annuria Fithri, Najma Annuria Narsito Narsito Neza Rahayu Niken Oktora Niken Oktora Nirwan Syarif Normah Normah Normah Normah, Normah Nova Yuliasari Novie Juleanti Novie Juleanti Novie Juleanti Nur Ahmad Nur Ahmad, Nur Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nurlisa Hidayati Nur’aini, Siti Nyanyu Ummu Hani Palita Tamba Patimah Mega Syah Bahar Nur Siregar Patimah Mega Syah Bahar Nur Siregar Patimah Mega Syah Bahar Nur Siregar Poedji Loekitowati Hariani Putri Erlyn Putri, Bunga Indah R.A. Mika Melviana Rabelia Juladika Sayeri Radja Nardo Purba Rakhmawati Farma Ramadhan, Jeri Rananda Vinsiah Randi O. Saragih Ratna, L.P Ratna, L.P Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risfidian Mohadi Risma Kurniawati M Rohmatullaili Rohmatullaili, Rohmatullaili Roy Andreas Sabat Okta Ceria Sitompul, Sabat Okta Ceria Samat Samat Savira, Dila Setiawan Yusuf Setiawati Yusuf Setiawati Yusuf Sherly Agustina, Sherly Siregar, Patimah Mega Syah Bahar Nur Sitanggang, Jonra P. Soerya, Balada Sri Juari Santosa Suheryanto Suheyanto Suheryanto Sumiati Sumiati SUMIATI, Susila Arita Syaflina Lamin Syafrina Lamin, Syafrina Tamizi Taher Tarmizi Taher Welinda Me Wibiyan, Sahrul Wijaya, Alfan Winda Fitriana Yeni Iswanti Yoshinori Yamanoi Yosi Saria Yosi Saria Yosi Saria Yosine Susi Yosine Susie Yunita Irianty Zahara, Zaqiya Artha Zazili Hanafiah Zultriana