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Journal : Journal of Applied Materials and Technology

 1 
Photo-Fenton of Dyes Degradation Using Covalent Triazine Frameworks: Toward Industrial Wastewater Treatment Applications Prawiranegara, Barata Aditya; Sugesti, Heni; Suhendri; Abid, Hussein Rasool; Azhar, Muhammad Rizwan; Rada, Zana Hassan; Manawan, Maykel; Utama, Panca Setia
Journal of Applied Materials and Technology Vol. 5 No. 2 (2024): March 2024
Publisher : Faculty of Engineering Universitas Riau and Applied Materials and Technology Society

Show Abstract | Download Original | Original Source | Check in Google Scholar | DOI: 10.31258/Jamt.5.2.77-85

Abstract

A Covalent Triazine Framework (CTF-1) and carbon nanospheres (CS) were synthesized to develop a porous, thermally stable, and efficient photocatalyst for dye degradation in wastewater treatment applications. The synthesized composite material exhibited a high surface area exceeding 400 m²/g, a well-defined mesoporous structure, and excellent optical properties, including strong light absorption extending up to 550 nm and a moderate band gap of approximately 2.8 eV. These characteristics promote effective visible light-driven photocatalysis. The photocatalytic performance was assessed by degrading methylene blue (MB) as a model organic dye pollutant under photo-Fenton conditions. The system demonstrated high efficiency, with over 90% of the dye removed within 120 minutes of irradiation. The degradation followed pseudo-first-order kinetics, confirming the photocatalytic nature of the reaction. Parameter studies indicated that hydroxyl radicals (•OH) were the dominant reactive species responsible for dye degradation. Moreover, CTF-1 retained its photocatalytic activity and structural integrity over multiple reuse cycles, showcasing excellent reusability and stability. The integration of high surface area for dye adsorption, efficient photoactivation under visible light, and robust radical generation synergistically contributed to the enhanced degradation performance. The study highlights the promising role of CTF-1 and its composites as multifunctional materials for advanced oxidation processes. Given its effectiveness, durability, and environmental compatibility, CTF-1 presents a sustainable and scalable solution for the treatment of dye-laden industrial wastewater. This work contributes to the development of next-generation photocatalysts aimed at addressing global challenges in water pollution and environmental remediation.
Co-Authors Abdhillah, Anzalini Abdurahman, Dede Abid, Hussein Rasool Ade Onny Siagian Agus Ismail Ahmad Fadli Ahmad Zaky, Ahmad Akbar, Nova Nauval Al Fauzi, Muhamad Iqbal Alel, Ariya Eka Alltop Amri Ya Habib Al’farisi, Cory Dian Amir Rofiudin Ani Ardian Kusmahardhika Ary Agung Wibowo Awaluddin Azhar, Muhammad Rizwan Bachtarino Bahrul Ulum Baihaqi, Wildan Budiati, Sekar Chairun Nisa Chrisca Lolita De Tian Septiana Sopandi Deffy Susanti Denny Martin Didin, Dede Ediyanto Eka Altiarika Ellya Rakhmawati Faisal Ahmad Fandila, Thasya Umy Fauziah, Nadia Kurnia Fendy Ferdy Ashari Syawal Fernanda Putra Adela Fikri Fahrudin Friti May Sandi Hanif Aulawi HARIS MUNANDAR Harun Sujadi Hastuti, Ririn Puji Haudi Helena, Dida Hendra Raza Heru Wahyu Herwanto Hidayatullah, Aldi Ibrahim N S Iis Khurniati Ikhyanuddin Indah Waraswita INDRA KESUMA NASUTION Ira Rizka Aisyah Lubis Irva Widiyawati Julius Kayne Karmelita, Mita Karmila, Mita Khusniyati Masykuroh Khusnul Muttaqiyah Koerniawan, M. Donny Lolita, Chrisca Luhur Adi Prasetya Manawan, Maykel Maryanah, Sri Meyke Garzia, Meyke Muhamaad Janwar Muhammad Ardian Muhammad Aris Ichwanto Muhammad Azhar Fahrezi Mutamima, Anisa N Ginting Nida, Milhatun Norimune, Kawai Nunu Nurdiana Nurazizah, Riri Nurfatihayati Nurjama’yah br Ketaren Nurul Aurila Mafaza Pahrudin Pikih Alpahri Prawiranegara, Barata Aditya Putri Indriyani Rada, Zana Hassan Rahmansyah Ranny Anggraeni Rahmawardani Reimond Hassangapan Mikkael Rian Syahmulloh Hendranawan Richnady, William Rico Nur Ilham Rohastono Ajie Ruswandi, Uus Salsabila Thifal Nabil Haq Samodra, Joko Satria, Doni Shilpana Anjelika Siti Ade Ida Rosia Sri Rahayu Sanusi Sugesti, Heni Sumringah, Mada SUNARNO Suwandi Tai, Calvin Tri Suyati Utama, Panca Setia Vanny Aulia Wendy Yansah WIJOYO, HADION Wiwik Kusdaryani Yelmida Azis Yolanda, Yogi Zalsahra, Rendy